Path integral Monte Carlo calculation of electronic forces

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Path integral Monte Carlo calculation of electronic forces

We describe a method to evaluate electronic forces by path integral Monte Carlo ~PIMC! calculation. Electronic correlations, as well as thermal effects, are included naturally in this method. For fermions, a restricted approach is used to avoid the ‘‘sign’’ problem. The PIMC force estimator is local and has a finite variance. We applied this method to determine the bond length of H2 and the che...

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ژورنال

عنوان ژورنال: Physical Review E

سال: 1998

ISSN: 1063-651X,1095-3787

DOI: 10.1103/physreve.58.5123